Lotso

Scroop

Edit: Scroop is unique among Pure Evils in that he passes the Moral Event Horizon by sending someone into the literal event horizon of a black hole.

Dr. Facilier. His scene of offering the "wayward" souls to his friends

@GlitchProductionsFan

What about when he stomped Ray to death?

Generic kill the heroes villainy

Odalia was for the most generic abusive parent and weapons dealer, but her giving Belos a vital resource for his genocide campaign knowing full well the consequences was what allowed her to pass the heinous standard.